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Corrosion investigations on zircaloy-4 and titanium dissolver materials for MOX fuel dissolution in concentrated nitric acid containing fluoride ions
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2016 (English)In: Journal of Nuclear Materials, ISSN 0022-3115, E-ISSN 1873-4820, Vol. 473, p. 157-166Article in journal (Refereed) Published
Abstract [en]

Aqueous reprocessing of plutonium-rich mixed oxide fuels require fluoride as a dissolution catalyst in boiling nitric acid for an effective dissolution of the spent fuel. High corrosion rates were obtained for the candidate dissolver materials zircaloy-4 (Zr-4) and commercial pure titanium (CP-Ti grade 2) in boiling 11.5 M HNO3 + 0.05 M NaF. Complexing the fluoride ions either with Al(NO3)3 or ZrO(NO3)2 aided in decreasing the corrosion rates of Zr-4 and CP-Ti. From the obtained corrosion rates it is concluded that CP-Ti is a better dissolver material than Zr-4 for extended service life in boiling 11.5 M HNO3+0.05 M NaF, when complexed with 0.15 M ZrO(NO3)2. XPS analysis confirmed the presence of TiO2 and absence of fluoride on the surface of CP-Ti samples, indicating that effective complexation had occurred in solution leading to passivation of the metal and imparting high corrosion resistance.

Place, publisher, year, edition, pages
2016. Vol. 473, p. 157-166
Keywords [en]
Zircaloy, Titanium, Nitric acid, Passivation, Fluoride, Dissolution, Complexing ions
National Category
Materials Engineering
Identifiers
URN: urn:nbn:se:du-31399DOI: 10.1016/j.jnucmat.2016.02.018OAI: oai:DiVA.org:du-31399DiVA, id: diva2:1381204
Available from: 2019-12-20 Created: 2019-12-20 Last updated: 2019-12-20Bibliographically approved

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Publisher's full texthttp://www.sciencedirect.com/science/article/pii/S0022311516300484

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Jayamani, Jayaraj

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CiteExportLink to record
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  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • chicago-author-date
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  • Other style
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  • de-DE
  • en-GB
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  • nn-NO
  • nn-NB
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